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  1. 原著論文

Rayleigh Scattering of Synchrotron Mössbauer Radiation using a Variable Bandwidth Nuclear Bragg Monochromator

https://repo.qst.go.jp/records/86061
https://repo.qst.go.jp/records/86061
a0aec3ab-5a1a-4a2a-a8fc-79c108f15915
Item type 学術雑誌論文 / Journal Article(1)
公開日 2022-04-06
タイトル
タイトル Rayleigh Scattering of Synchrotron Mössbauer Radiation using a Variable Bandwidth Nuclear Bragg Monochromator
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_6501
資源タイプ journal article
アクセス権
アクセス権 metadata only access
アクセス権URI http://purl.org/coar/access_right/c_14cb
著者 Takaya, Mitsui

× Takaya, Mitsui

WEKO 1049020

Takaya, Mitsui

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Masuda, Ryo

× Masuda, Ryo

WEKO 1049021

Masuda, Ryo

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Kitao, Shinji

× Kitao, Shinji

WEKO 1049022

Kitao, Shinji

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Kobayashi, Yasuhiro

× Kobayashi, Yasuhiro

WEKO 1049023

Kobayashi, Yasuhiro

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Makoto, Seto

× Makoto, Seto

WEKO 1049024

Makoto, Seto

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Takaya, Mitsui

× Takaya, Mitsui

WEKO 1049025

en Takaya, Mitsui

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Makoto, Seto

× Makoto, Seto

WEKO 1049026

en Makoto, Seto

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抄録
内容記述タイプ Abstract
内容記述 By combining a variable bandwidth nuclear Bragg monochromator and a nuclear resonant reference absorber, a spectroscopic method using Rayleigh scattering of synchrotron Mössbauer radiation has been successfully developed. The nuclear Bragg monochromator filters single-line 57Fe-Mössbauer radiation with variable energy bandwidth in the range of 10-8 to 10-6 eV from broadband synchrotron radiation, while the reference absorber acts as an energy analyzer for the scattered radiation by the sample that contains no Mössbauer isotope. By optimizing the energy bandwidth of the Mössbauer radiation and selecting the appropriate nuclear resonant absorber, it is possible to separate elastic and inelastic scattering components from the scattered radiation, and also to measure the ultrahigh energy resolution inelastic X-ray scattering spectrum in the wide dynamic range. This paper describes the principle and experimental system of this method, and the first feasible applications including the observations of glass transition of polystyrenes with different molecular weights and quasi-elastic scattering spectra of liquid glycerol are shown. The results clearly demonstrate that the developed method is suitable for studying the molecular dynamics in soft matter and paves the way for new applications of non-Mössbauer experiments using a nuclear Bragg monochromator.
書誌情報 Journal of the Physical Society of Japan

巻 91, p. 064001-1-064001-8, 発行日 2022-04
出版者
出版者 Journal of the Physical Society of Japan
ISSN
収録物識別子タイプ ISSN
収録物識別子 0031-9015
DOI
識別子タイプ DOI
関連識別子 10.7566/JPSJ.91.064001
関連サイト
識別子タイプ DOI
関連識別子 https://doi.org/10.7566/JPSJ.91.064001
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