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Temporal trend of 240Pu/239Pu atom ratios in water columns in the western North Pacific Ocean and its marginal seas
https://repo.qst.go.jp/records/84435
https://repo.qst.go.jp/records/8443598cb5f5d-c967-45ef-9ff1-b8644164122a
| Item type | 学術雑誌論文 / Journal Article(1) | |||||
|---|---|---|---|---|---|---|
| 公開日 | 2021-06-25 | |||||
| タイトル | ||||||
| タイトル | Temporal trend of 240Pu/239Pu atom ratios in water columns in the western North Pacific Ocean and its marginal seas | |||||
| 言語 | ||||||
| 言語 | eng | |||||
| 資源タイプ | ||||||
| 資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
| 資源タイプ | journal article | |||||
| アクセス権 | ||||||
| アクセス権 | metadata only access | |||||
| アクセス権URI | http://purl.org/coar/access_right/c_14cb | |||||
| 著者 |
Yamada, Masatoshi
× Yamada, Masatoshi× Zheng, Jian× Zheng, Jian |
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| 抄録 | ||||||
| 内容記述タイプ | Abstract | |||||
| 内容記述 | The 240Pu/239Pu atom ratios were determined by inductively coupled plasma mass spectrometry for seawater samples from the Okinawa Trough in the western North Pacific Ocean margin to identify their Pu sources and to elucidate the temporal variability in atom ratios in the water columns in the western North Pacific Ocean and its marginal seas. The 239Pu, 240Pu and 239+240Pu inventories were 12.2 ± 0.5, 10.5 ± 0.5 and 22.7 ± 1.0 Bq m-2, respectively. The observed 240Pu/239Pu ratios were clearly greater than the mean global fallout ratio of ~0.18 with a mean value of 0.236 ± 0.014. The observed greater atom ratios confirmed the presence of close-in fallout Pu from nuclear testing at the Pacific Proving Grounds (PPG). The relative percentage of the PPG-derived Pu to global fallout Pu was estimated as 41 ± 10%. The water column 239+240Pu inventory originating from the PPG close-in fallout was also calculated as 9.2 ± 0.4 Bq m-2. The temporal variability in the mean 240Pu/239Pu atom ratios in the water columns in the western North Pacific Ocean and its marginal seas was obtained through comparison of the present study values and the previously reported values, and it had no significant temporal variation with a mean value of 0.237 ± 0.004 during the observation period of 1984-2015. The 239Pu and 240Pu derived from the two different sources of global fallout and the close-in fallout at the PPG were homogenized in the water masses in the studied areas. | |||||
| 書誌情報 |
Journal of Environmental Radioactivity 巻 240, p. 106737, 発行日 2021-09 |
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| 出版者 | ||||||
| 出版者 | Elsevier | |||||
| ISSN | ||||||
| 収録物識別子タイプ | ISSN | |||||
| 収録物識別子 | 0265-931X | |||||
| DOI | ||||||
| 識別子タイプ | DOI | |||||
| 関連識別子 | 10.1016/j.jenvrad.2021.106737 | |||||
| 関連サイト | ||||||
| 識別子タイプ | URI | |||||
| 関連識別子 | https://www.sciencedirect.com/science/article/pii/S0265931X21002095 | |||||
