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  1. 原著論文

Background and fingerprint characteristics of anthropogenic 236U and137Cs in soil and road dust samples collected from Beijing and Zhangjiakou, China

https://repo.qst.go.jp/records/80331
https://repo.qst.go.jp/records/80331
ab5f3e95-c92e-4e5d-91d4-7f729d6cc377
Item type 学術雑誌論文 / Journal Article(1)
公開日 2020-08-17
タイトル
タイトル Background and fingerprint characteristics of anthropogenic 236U and137Cs in soil and road dust samples collected from Beijing and Zhangjiakou, China
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_6501
資源タイプ journal article
アクセス権
アクセス権 metadata only access
アクセス権URI http://purl.org/coar/access_right/c_14cb
著者 Shao, Yang

× Shao, Yang

WEKO 883000

Shao, Yang

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Yang, Guosheng

× Yang, Guosheng

WEKO 883001

Yang, Guosheng

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Min, Luo

× Min, Luo

WEKO 883002

Min, Luo

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Xu, Diandou

× Xu, Diandou

WEKO 883003

Xu, Diandou

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Tazoe, Hirofumi

× Tazoe, Hirofumi

WEKO 883004

Tazoe, Hirofumi

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Yamada, Masatoshi

× Yamada, Masatoshi

WEKO 883005

Yamada, Masatoshi

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Ma, Lingling

× Ma, Lingling

WEKO 883006

Ma, Lingling

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Yang, Guosheng

× Yang, Guosheng

WEKO 883007

en Yang, Guosheng

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抄録
内容記述タイプ Abstract
内容記述 236U has attracted more attention as an environmental tracer in recent years. However, in-depth study of 236U in terrestrial environments is still rare in China. Data on 236U and 137Cs concentrations in soil and road dust samples collected from Beijing and Zhangjiakou, China were obtained to demonstrate the background and distinct characteristics of anthropogenic 236U and 137Cs. 236U and 137Cs were detected in the range of (1.10–7.90)×107 atoms g-1 and below the method limits of detection to 5.30 Bq kg-1. A clear characteristic was observed in road dust, where 236U concentrations increased with decreasing of sample particle size. Soil samples showed an irregular characteristic, but the highest 236U concentrations were observed in particle size fraction of < 0.053 mm in both samples. This phenomenon was caused by U chemical properties, higher specific surface areas and organic compounds in fine particles. Anthropogenic radionuclides fingerprint characteristics in < 0.053 mm samples were specially discussed. 236U/238U atom ratios were detected in the range of (0.627–3.38)×10-8. A weak correlation between anthropogenic 236U and natural U isotopes were observed. The intermediate correlation between 236U and 137Cs indicated somewhat distinct migration behavior of these two radionuclides in soil after release to the environment. The released amount of 236U from global fallout during the period of atmospheric nuclear weapons testing was roughly estimated to be 1300±448 kg. These results could be used as fingerprint information for anthropogenic 236U migration behavior and tracer application in environment.
書誌情報 Chemosphere

巻 263, 発行日 2020-08
ISSN
収録物識別子タイプ ISSN
収録物識別子 0045-6535
DOI
識別子タイプ DOI
関連識別子 10.1016/j.chemosphere.2020.127909
関連サイト
識別子タイプ URI
関連識別子 https://www.sciencedirect.com/science/article/abs/pii/S0045653520321044
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