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Background and fingerprint characteristics of anthropogenic 236U and137Cs in soil and road dust samples collected from Beijing and Zhangjiakou, China
https://repo.qst.go.jp/records/80331
https://repo.qst.go.jp/records/80331ab5f3e95-c92e-4e5d-91d4-7f729d6cc377
Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2020-08-17 | |||||
タイトル | ||||||
タイトル | Background and fingerprint characteristics of anthropogenic 236U and137Cs in soil and road dust samples collected from Beijing and Zhangjiakou, China | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
アクセス権 | ||||||
アクセス権 | metadata only access | |||||
アクセス権URI | http://purl.org/coar/access_right/c_14cb | |||||
著者 |
Shao, Yang
× Shao, Yang× Yang, Guosheng× Min, Luo× Xu, Diandou× Tazoe, Hirofumi× Yamada, Masatoshi× Ma, Lingling× Yang, Guosheng |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | 236U has attracted more attention as an environmental tracer in recent years. However, in-depth study of 236U in terrestrial environments is still rare in China. Data on 236U and 137Cs concentrations in soil and road dust samples collected from Beijing and Zhangjiakou, China were obtained to demonstrate the background and distinct characteristics of anthropogenic 236U and 137Cs. 236U and 137Cs were detected in the range of (1.10–7.90)×107 atoms g-1 and below the method limits of detection to 5.30 Bq kg-1. A clear characteristic was observed in road dust, where 236U concentrations increased with decreasing of sample particle size. Soil samples showed an irregular characteristic, but the highest 236U concentrations were observed in particle size fraction of < 0.053 mm in both samples. This phenomenon was caused by U chemical properties, higher specific surface areas and organic compounds in fine particles. Anthropogenic radionuclides fingerprint characteristics in < 0.053 mm samples were specially discussed. 236U/238U atom ratios were detected in the range of (0.627–3.38)×10-8. A weak correlation between anthropogenic 236U and natural U isotopes were observed. The intermediate correlation between 236U and 137Cs indicated somewhat distinct migration behavior of these two radionuclides in soil after release to the environment. The released amount of 236U from global fallout during the period of atmospheric nuclear weapons testing was roughly estimated to be 1300±448 kg. These results could be used as fingerprint information for anthropogenic 236U migration behavior and tracer application in environment. | |||||
書誌情報 |
Chemosphere 巻 263, 発行日 2020-08 |
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ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 0045-6535 | |||||
DOI | ||||||
識別子タイプ | DOI | |||||
関連識別子 | 10.1016/j.chemosphere.2020.127909 | |||||
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識別子タイプ | URI | |||||
関連識別子 | https://www.sciencedirect.com/science/article/abs/pii/S0045653520321044 |