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Analytical method development of Sr-90 measurement in soil samples affected by the Fukushima nuclear accident

https://repo.qst.go.jp/records/65541
https://repo.qst.go.jp/records/65541
387cef8e-a766-4a6f-9be0-01b83522be54
Item type 会議発表用資料 / Presentation(1)
公開日 2014-11-25
タイトル
タイトル Analytical method development of Sr-90 measurement in soil samples affected by the Fukushima nuclear accident
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_c94f
資源タイプ conference object
アクセス権
アクセス権 metadata only access
アクセス権URI http://purl.org/coar/access_right/c_14cb
著者 Nor, Kavasi

× Nor, Kavasi

WEKO 1038723

Nor, Kavasi

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Sarata Kumar, Sahoo

× Sarata Kumar, Sahoo

WEKO 1038724

Sarata Kumar, Sahoo

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Arae, Hideki

× Arae, Hideki

WEKO 1038725

Arae, Hideki

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Aono, Tatsuo

× Aono, Tatsuo

WEKO 1038726

Aono, Tatsuo

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Yoshida, Satoshi

× Yoshida, Satoshi

WEKO 1038727

Yoshida, Satoshi

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Kavasi, Norbert

× Kavasi, Norbert

WEKO 1038728

en Kavasi, Norbert

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Sahoo, Sarata

× Sahoo, Sarata

WEKO 1038729

en Sahoo, Sarata

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Hideki, Arae

× Hideki, Arae

WEKO 1038730

en Hideki, Arae

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Tatsuo, Aono

× Tatsuo, Aono

WEKO 1038731

en Tatsuo, Aono

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Satoshi, Yoshida

× Satoshi, Yoshida

WEKO 1038732

en Satoshi, Yoshida

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抄録
内容記述タイプ Abstract
内容記述 There is an increasing interest on Sr-90 measurement in environmental samples after the Fukushima Daiichi nuclear power plant (FDNPP) accident since it is a bone seeker isotope with high toxicity. Radioactive strontium, cesium and plutonium isotopes are the main contributors of radioactive contamination for many years after FDNPP accident due to their longer half-life. Radiocesium (Cs-137, Cs-134) deposition is significantly high over a large area in Japan owing to the FDNPP accident. Consequently, the presence of radiocesium in environmental samples collected from contaminated fields is obvious.
Sr-90 is a pure beta emitter radionuclide thus separation from self-absorptive sample matrix and other disturbing beta emitter radionuclides is required. Most of the Sr-90 separation methods are based on precipitation, liquid-liquid extraction, ion-exchange chromatography and extraction chromatography. Recently extraction chromatography using selective Sr resin is the most popular method since it is easy to handle and simple to use. Disadvantages of the Sr resin, such as strontium retention decrement in the presence of elevated amount of calcium, high lead and tetravalent actinides retention are well known and overcome.
In our work, Sr-90 specific activity were analysed in soil samples affected by FDNPP accident. Each sample had elevated radiocesium specific activity, the average of Cs-134 was 46 (5.5-120) Bq/g while the average of Cs-137 was 91 (11-230) Bq/g, respectively. The perfect separation of radiocesium from Sr-90 is a cardinal point to gain accurate Sr-90 result as the radiocesium also undergoes beta decay emitting gamma-rays. Furthermore, there is another problem, i.e. of high iron concentration in Japanese soils.
In our laboratory, an efficient separation procedure was established to remove radiocesium and iron from soil samples to produce required samples for a liquid scintillation counter. In addition to radiometric detection methods, mass spectrometric methods show excellent prospects in nuclear measurements techniques. Thus, separation procedure development has been aimed for thermal ionization mass spectrometry.
会議概要(会議名, 開催地, 会期, 主催者等)
内容記述タイプ Other
内容記述 The 9th International Symposium on the Matural Radiation Environment(NRE-IX)
発表年月日
日付 2014-09-24
日付タイプ Issued
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