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Enrichment of ODMR-active nitrogen-vacancy centres in five-nanometre-sized detonation-synthesized nanodiamonds: Nanoprobes for temperature, angle and position.
https://repo.qst.go.jp/records/49398
https://repo.qst.go.jp/records/4939864edaef7-35a3-41fd-b046-0e2a8feb78ff
Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2018-04-06 | |||||
タイトル | ||||||
タイトル | Enrichment of ODMR-active nitrogen-vacancy centres in five-nanometre-sized detonation-synthesized nanodiamonds: Nanoprobes for temperature, angle and position. | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
アクセス権 | ||||||
アクセス権 | metadata only access | |||||
アクセス権URI | http://purl.org/coar/access_right/c_14cb | |||||
著者 |
Sotoma, Shingo
× Sotoma, Shingo× Terada, Daiki× F. Segawa, Takuya× Igarashi, Ryuji× Harada, Yoshie× Shirakawa, Masahiro× Igarashi, Ryuji× Harada, Yoshie |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | The development of sensors to estimate physical properties, and their temporal and spatial variation, has been a central driving force in scientific breakthroughs. In recent years, nanosensors based on quantum measurements, such as nitrogen-vacancy centres (NVCs) in nanodiamonds, have been attracting much attention as ultrastable, sensitive, accurate and versatile physical sensors for quantitative cellular measurements. However, the nanodiamonds currently available for use as sensors have diameters of several tens of nanometres, much larger than the usual size of a protein. Therefore, their actual applications remain limited. Here we show that NVCs in an aggregation of 5-nm-sized detonation-synthesized nanodiamond treated by Krüger's surface reduction (termed DND-OH) retains the same characteristics as observed in larger diamonds. We show that the negative charge at the NVC are stabilized, have a relatively long T2 spin relaxation time of up to 4 μs, and are applicable to thermosensing, one-degree orientation determination and nanometric super-resolution imaging. Our results clearly demonstrate the significant potential of DND-OH as a physical sensor. Thus, DND-OH will raise new possibilities for spatiotemporal monitoring of live cells and dynamic biomolecules in individual cells at single-molecule resolution. | |||||
書誌情報 |
Scientific Reports 巻 8, 号 1, p. 5463, 発行日 2018-04 |
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出版者 | ||||||
出版者 | Nature Publishing Group | |||||
ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 2045-2322 | |||||
DOI | ||||||
識別子タイプ | DOI | |||||
関連識別子 | 10.1038/s41598-018-23635-5 | |||||
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識別子タイプ | URI | |||||
関連識別子 | https://www.nature.com/articles/s41598-018-23635-5 |