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Investigation of hydrogen generation from the reaction of beryllium pebbles with water vapor for WCCB-TBM

https://repo.qst.go.jp/records/2001161
https://repo.qst.go.jp/records/2001161
e32fbd76-f5be-46f4-907f-d8c72e9a83a7
アイテムタイプ 学術雑誌論文 / Journal Article(1)
公開日 2024-04-17
タイトル
タイトル Investigation of hydrogen generation from the reaction of beryllium pebbles with water vapor for WCCB-TBM
言語 en
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_6501
資源タイプ journal article
著者 Koga Yuki

× Koga Yuki

Koga Yuki

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Jaehwan Kim

× Jaehwan Kim

Jaehwan Kim

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Ohta Yuga

× Ohta Yuga

Ohta Yuga

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Kawamura Yoshinori

× Kawamura Yoshinori

Kawamura Yoshinori

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Nakamichi Masaru

× Nakamichi Masaru

Nakamichi Masaru

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Hirose Takanori

× Hirose Takanori

Hirose Takanori

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抄録
内容記述タイプ Abstract
内容記述 Be pebble, as a neutron multiplier material, is being explored for the development of a Water-Cooled Ceramic Breeder Test Blanket Module (WCCB-TBM) in Japan for the International Thermonuclear Experiment Reactor (ITER) project. The Be pebbles were fabricated by the rotating electrode process (REP). However, as the safety of the test blanket module (TBM) could be compromised by hydrogen generation via Be?H2O reaction owing to the leakage of pressurized water from the cooling pipes inside TBM, the safety assessment of TBM must be conducted using the Be?H2O reactivity data for the Be pebbles whose fabrication method is the same as that for TBM (i.e., REP). Thus, in this study, a Be?H2O reactivity test was conducted using Be pebbles that were fabricated by REP to characterize the generated hydrogen and evaluate the hydrogen generation (HG) rates toward WCCB-TBM safety assessment. First, the Be?H2O reactivity data were obtained at ? 300 °C (the coolant temperature for the TBM). The experimental results and oxidation rate of the Be pebbles revealed that only the Be surface may have been oxidized at 300 °C?600 °C, although its inside was oxidized at 700 °C?1000 °C. Further, the experimental data?derived HG rates at 300 °C?1000 °C increased with the temperature and the tendency changed in the three temperature regions. The HG rates did not contradict those reported by previous studies. Additionally, these regions corresponded to each expected Be?H2O reaction behavior at 300 °C?1000 °C. At a Be temperature of < 600 °C, the generated hydrogen from TBM will not exceed 2.5 kg of a limitation by the water leakage on the estimation based on the HG rates and the qualitative effects of the safety functions.
書誌情報 Nuclear Materials and Energy

巻 39, p. 101642, 発行日 2024-03
出版者
出版者 Elsevier
DOI
識別子タイプ DOI
関連識別子 https://doi.org/10.1016/j.nme.2024.101642
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