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  1. 原著論文

Dynamic Jahn-Teller effect in the strong spin-orbit coupling regime

https://repo.qst.go.jp/records/2000918
https://repo.qst.go.jp/records/2000918
88707c01-a3c4-42fc-bec2-14e4be93c2da
アイテムタイプ 学術雑誌論文 / Journal Article(1)
公開日 2024-10-08
タイトル
タイトル Dynamic Jahn-Teller effect in the strong spin-orbit coupling regime
言語 en
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_6501
資源タイプ journal article
著者 Ivica Zivkovic

× Ivica Zivkovic

Ivica Zivkovic

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Jian-Rui Soh

× Jian-Rui Soh

Jian-Rui Soh

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Oleg Malanyuk

× Oleg Malanyuk

Oleg Malanyuk

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Ravi Yadav

× Ravi Yadav

Ravi Yadav

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Federico Pisani

× Federico Pisani

Federico Pisani

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Aria M. Tehrani

× Aria M. Tehrani

Aria M. Tehrani

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Davor Tolj

× Davor Tolj

Davor Tolj

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Jana Pasztorova

× Jana Pasztorova

Jana Pasztorova

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Daigorou Hirai

× Daigorou Hirai

Daigorou Hirai

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Yuan Wei

× Yuan Wei

Yuan Wei

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Wenliang Zhang

× Wenliang Zhang

Wenliang Zhang

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Carlos Galdino

× Carlos Galdino

Carlos Galdino

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Tianlun Yu

× Tianlun Yu

Tianlun Yu

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Kenji Ishii

× Kenji Ishii

Kenji Ishii

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Albin Demuer

× Albin Demuer

Albin Demuer

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Oleg V. Yazyev

× Oleg V. Yazyev

Oleg V. Yazyev

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Thorsten Schmitt

× Thorsten Schmitt

Thorsten Schmitt

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Henrik M. Ronnow

× Henrik M. Ronnow

Henrik M. Ronnow

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抄録
内容記述タイプ Abstract
内容記述 Exotic quantum phases, arising from a complex interplay of charge, spin, lat- tice and orbital degrees of freedom, are of immense interest to a wide research community. A well-known example of such an entangled behavior is the Jahn- Teller effect, where the lifting of orbital degeneracy proceeds through lattice distortions. Here we demonstrate that a highly-symmetrical 5d1 double per- ovskite Ba2MgReO6, comprising a 3D array of isolated ReO6 octahedra, represents a rare example of a dynamic Jahn-Teller system in the strong spin- orbit coupling regime. Thermodynamic and resonant inelastic x-ray scattering experiments, supported by quantum chemistry calculations, undoubtedly show that the Jahn-Teller instability leads to a ground-state doublet, resolving a long-standing puzzle in this family of compounds. The dynamic state of ReO6 octahedra persists down to the lowest temperatures, where a multipolar order sets in, allowing for investigations of the interplay between a dynamic JT effect and strongly correlated electron behavior.
書誌情報 Nature communications

巻 15, p. 8587, 発行日 2024-10
出版者
出版者 Springer Nature
ISSN
収録物識別子タイプ ISSN
収録物識別子 2041-1723
DOI
識別子タイプ DOI
関連識別子 10.1038/s41467-024-52935-w
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