@article{oai:repo.qst.go.jp:00048691, author = {湊, 太志 and 塚田, 和明 and 佐藤, 望 and 渡辺, 智 and 佐伯, 秀也 and 川端, 方子 and 橋本, 慎太郎 and 永井, 泰樹 and 塚田 和明 and 渡辺 智 and 佐伯 秀也 and 川端 方子 and 永井 泰樹}, issue = {11}, journal = {Journal of the Physical Society of Japan (JPSJ)}, month = {Nov}, note = {We, for the first time, measured the yield of 99Mo, the mother nuclide of 99mTc used in nuclear medicine diagnostic procedures, produced by the 100Mo(n,2n)99Mo reaction with accelerator neutrons. The neutrons with a continuous energy spectrum from the thermal energy up to about 40MeV were provided by the C(d,n) reaction with 40MeV deuteron beams. It was proved that the 99Mo yield agrees with that estimated by using the latest data on neutrons from the C(d,n) reaction and the evaluated cross section of the 100Mo(n,2n)99Mo reaction given in the Japanese Evaluated Nuclear Data Library. On the basis of the agreement, a systematic calculation was carried out to search for an optimum condition that enables us to produce as much 99Mo as possible with a good 99Mo=100Mo value from an economical point of view. The calculated 99Mo yield from a 150 g 100MoO3 sample indicated that about 30% of the demand for 99Mo in Japan can be met with a single accelerator capable of 40 MeV, 2mA deuteron beams. Here, by referring to an existing 18F- fluorodeoxyglucose (FDG) distribution system we assumed that 99mTc radiopharmaceuticals formed after separating 99mTc from 99Mo can be delivered to hospitals from a radiopharmaceutical company within 6 h. The elution of 99mTc from 99Mo twice a day would meet about 50% of the demand for 99Mo.}, pages = {114803-1--114803-6}, title = {Measurement and Estimation of the 99Mo Production Yield by 100Mo(n,2n)99Mo}, volume = {86}, year = {2017} }