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Wetting induced oxidation of Pt-based nano catalysts revealed by in situ high energy resolution X-ray absorption spectroscopy
https://repo.qst.go.jp/records/48453
https://repo.qst.go.jp/records/48453a2dda4ea-68a8-4266-ae1c-feb33a3bbe3e
Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2018-02-06 | |||||
タイトル | ||||||
タイトル | Wetting induced oxidation of Pt-based nano catalysts revealed by in situ high energy resolution X-ray absorption spectroscopy | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
アクセス権 | ||||||
アクセス権 | metadata only access | |||||
アクセス権URI | http://purl.org/coar/access_right/c_14cb | |||||
著者 |
Cui, Yitao
× Cui, Yitao× Harada, Yoshihisa× Niwa, Hideharu× Hatanaka, Tatsuya× Nakamura, Naoki× Ando, Masaki× Yoshida, Toyohiko× Ishii, Kenji× Matsumura, Daiju× Oji, Hiroshi× Ofuchi, Hironori× Oshima, Masaharu× 石井 賢司 |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | In situ high energy resolution fluorescence detection x-ray absorption spectroscopy (HERFD-XAS) was used to evaluate systematically the interactions of H2O and O2 adsorbed on Pt and Pt3Co nanoparticle catalysts in different sizes. The systematic increase in oxidation due to adsorption of different species (H2O adsorption < O2 adsorption < O2 + H2O coadsorption) suggests that cooperative behavior between O2 and H2O adsorptions is responsible for the overpotential induced by hydrated species in fuel cells. | |||||
書誌情報 |
Scientific Reports 巻 7, p. 1482-1-1482-8, 発行日 2017-05 |
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DOI | ||||||
識別子タイプ | DOI | |||||
関連識別子 | 10.1038/s41598-017-00639-1 | |||||
関連サイト | ||||||
識別子タイプ | URI | |||||
関連識別子 | https://www.nature.com/articles/s41598-017-00639-1 | |||||
関連名称 | https://www.nature.com/articles/s41598-017-00639-1 |