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Uranium and plutonium isotopes and their environmental implications in surface sediments from the Yangtze River catchment and estuary
https://repo.qst.go.jp/records/79934
https://repo.qst.go.jp/records/79934c24ba3ec-8780-4c92-a429-dd8e8a82fda2
Item type | 学術雑誌論文 / Journal Article(1) | |||||
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公開日 | 2020-05-07 | |||||
タイトル | ||||||
タイトル | Uranium and plutonium isotopes and their environmental implications in surface sediments from the Yangtze River catchment and estuary | |||||
言語 | ||||||
言語 | eng | |||||
資源タイプ | ||||||
資源タイプ識別子 | http://purl.org/coar/resource_type/c_6501 | |||||
資源タイプ | journal article | |||||
アクセス権 | ||||||
アクセス権 | metadata only access | |||||
アクセス権URI | http://purl.org/coar/access_right/c_14cb | |||||
著者 |
Liu, Zhiyong
× Liu, Zhiyong× Hu, Jun× Yamada, Masatoshi× Yang, Guosheng× Yang, Guosheng |
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抄録 | ||||||
内容記述タイプ | Abstract | |||||
内容記述 | The U-series and Pu isotope signatures in the environment have emerged as important tools for promoting geochemical studies. To enhance the understanding of U and Pu sources and behaviours in river systems, this study examined 234U, 235U, 236U, 238U and 239Pu, 240Pu isotopes in surface sediments collected from the Yangtze River catchment and estuary in China, for the first time. The 234U, 235U, 238U and 236U concentrations were measured in the range of 8.29–20.6 Bq/kg, 0.352–0.789 Bq/kg, 7.39–16.4 Bq/kg and (3.05–21.1) × 10 7 atoms/g. Additionally, the 236U/238U, 234U/238U and 235U/238U atom ratios were in the range of (1.43–6.85) × 10 −8 , (6.08–7.01) × 10 −5 and (7.49–8.08) × 10 −3 respectively. For all samples, the 239+240Pu activity concentrations ranged from 0.01 to 3.40 Bq/kg. In the Yangtze River catchment, 240Pu/ 239Pu atom ratios presented typical global fallout values (0.168–0.201); while in the Yangtze River estuary, higher values of 0.216–0.264 located between global fallout and PPG (Pacific Proving Grounds) close-in fallout values. From west to east, the 234U, 235U, 236U and 238U activities generally exhibited decreasing trend from the upstream parts of the river to the estuary. The values of 236U concentrations and 236U/238U, 240Pu/239Pu, 236U/239Pu atom ratios located in the range of global fallout level in environmental samples from other regions, therefore, it may be concluded that 236 U in surface sediments of the Yangtze River catchment and estuary are mainly derived from global fallout. |
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書誌情報 |
CATENA 巻 193, 発行日 2020-04 |
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出版者 | ||||||
出版者 | Elsevier | |||||
ISSN | ||||||
収録物識別子タイプ | ISSN | |||||
収録物識別子 | 0341-8162 | |||||
DOI | ||||||
識別子タイプ | DOI | |||||
関連識別子 | 10.1016/j.catena.2020.104605 | |||||
関連サイト | ||||||
識別子タイプ | DOI | |||||
関連識別子 | https://doi.org/10.1016/j.catena.2020.104605 |